The mountain range spanned at least 2,500 kilometres of modern west Africa and northeast Brazil, which at that time were part of the supercontinent Gondwana.
"Just like the Himalayas, this range was eroded intensely because it was so huge. As the sediments washed into the oceans they provided the perfect nutrients for life to flourish," said Professor Daniela Rubatto of the Research School of Earth Sciences at The Australian National University (ANU).
The discovery is the earliest evidence of Himalayan-scale mountains on Earth, scientists said.
"Although the mountains have long since washed away, rocks from their roots told the story of the ancient mountain range's grandeur," said co-researcher Professor Joerg Hermann.
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"The range was formed by two continents colliding. During this collision, rocks from the crust were pushed around 100 kilometres deep into the mantle, where the high temperatures and pressures formed new minerals," Hermann said.
Roots of the ancient mountain range, long since eroded, were found in Northeast Brazil.
Araujo recognised the samples were unique and brought the rocks to ANU where, using world-leading equipment, the research team accurately identified that the rocks were of similar age, and had been formed at similar, great depths.