"They're house hunting in London. Angie wants to slowly immerse herself in EU politics," a source said.
Though the parents of six toured a USD 39 million, seven-bedroom Westminster mansion in June, they are yet to buy it, reported Us magazine.
"It's a huge investment. Neither of them wants to throw down that amount of cash," the source said.
The couple were also in London in late June so that Jolie could attend a luncheon as part of her work on UK foreign policy and her ongoing campaign to end sexual violence in war crimes.