Best known for his satire, whimsy and observational jokes, Brand, 40, began his set last night by taking a potshot at his short- lived marriage to pop star Katy Perry. The couple had a lavish wedding in Rajasthan in 2010 only to divorce 14 months later.
"I have never performed in India, unless you call my marriage as a performance... In fact, there are a lot of Bollywood films that last longer than my marriage," Brand joked as he began his performance with a "Namaste".
The "Arthur" actor, while reading out a list of Bollywood celebrities he would like to be like, said he would try to seduce Deepika.
"The person I could potentially fall in love with and marry while I am in India, Deepika Padukone. She is popular. If by the end of the night I am not arrested or censored, we are going to look and see if I can perhaps seduce Deepika Padukone.
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"If anyone has her phone number, let me know, we can ring her in the course of the evening," he said.
"You people honk so much... As if devastation is coming. You are better when in an auditorium than on the road."
Brand will next be performing in Bengaluru (June 27) and Mumbai (June 28).