The 32-year-old and her football player husband, were spotted browsing luxury pads in the West Village area, reported New York Post.
The couple previously lived in the city, with Tom selling his Time Warner Center residence for a reported USD 17.5 million in 2011 and Bundchen accepting USD 4.4 million for her lavish town house.
She also received a staggering USD 12.95 million after moving out of her Barrow Street home in 2009.
They are currently dwelling in Los Angeles, which they share with their children Benjamin, three, and four-month-old Vivian, along with Tom's five-year-old son John from a previous relationship, was recently transformed to include a moat and bridge and a resort-style swimming pool in their back yard.
"We are excited to be using solar power as the main source of electricity in our home. And we are planting our own herbs, fruits and vegetables, which will be my favourite part of the house," she said.