Amit Kumar was also the mastermind of the multi-crore Gurgaon kidney racket in 2008 and was believed to have conducted over 500 illegal operations. The CBI had registered a case and an Interpol notice had been issued then for his arrest. Kumar was arrested in Nepal in February 2008.
The fresh racket was unearthed on September 11 in Gangotri charitable hospital in Lal Tappar area of rural Dehradun.
While Amit, Jeevan and Sarla were arrested from a parking lot in front of a hotel in sector 18, Panchkula in Haryana, Billu was arrested from Raiwala area in Dehradun, she said.
Rajiv Chaudhry is the man who ran the hospital after taking it on a lease.
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With these arrests the number of people held in connection with the case has risen to five.
A middleman named Javed was arrested on September 11.
Six mobile phones, a Mercedes and a BMW besides Rs 33.73 lakh in cash have been recovered from those arrested from Panchkula.
A car has also been recovered from Rajiv Chaudhry's driver Billu's possession, the SSP said.
It is being investigated whether transplant operations conducted illegally by Amit Kumar and Jeevan Kumar led to death of patients, the SSP said.