The 70-year-old president-elect, who has never previously held elective office, yesterday announced Oklahoma Attorney General Scott Pruitt, a climate skeptic, as environment chief and fast food executive Andy Puzder as labour secretary.
More than half his cabinet positions have now been filled, 43 days before the Republican is sworn in as the 45th president of the United States, the oldest man ever inaugurated into the office.
"I believe we're in the process of putting together one of the great cabinets that has ever been assembled in the history of our nation," Trump told a victory rally in Des Moines, Iowa.
"In filling my cabinet I'm looking for people who fully understand the meaning of service and who are committed to advancing the common good," he added, defending his appointment of a string of billionaires and millionaires.
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The incoming president triggered criticism by tapping a fossil fuel industry ally to head the Environmental Protection Agency (EPA) - outraging many who fear that he will reverse President Barack Obama's efforts to combat climate change.
In announcing the nomination of Pruitt - who will need Senate approval - Trump complained that "for too long," the EPA had spent "taxpayer dollars on an out-of-control anti- energy agenda that has destroyed millions of jobs."
Steny Hoyer, the number two Democrat in the House of Representatives, said Pruitt had spent years "fighting tooth and nail to help polluters erase or circumvent the critical environmental protections our nation has put in place."
Ken Kimmell, president of the Union of Concerned Scientists, described Pruitt as someone "on the outer extreme edge, and putting him in charge of EPA could really have devastating consequences."
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