The twin offensives are two of the most significant ground assaults against the extremists since they declared a self-styled "caliphate" in Iraq and Syria in 2014.
The assaults came as Syria's UN envoy said trapped civilians risk starvation unless Damascus and rebel groups allow greater access to humanitarian aid convoys.
Near the front line north of Raqa city, an AFP photographer saw US soldiers yesterday assisting a Kurdish-dominated alliance known as the Syrian Democratic Forces.
It said its fighters had "advanced seven kilometres from Ain Issa and liberated five villages and four fields."
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"We liberated the villages of Fatisah, Namroudiya, and Wastah as well as several fields. The coming battle will hold a lot of big surprises," SDF field commander Baraa al-Ghanem told AFP.
The Syrian Observatory for Human Rights said SDF fighters on Thursday were shelling IS positions near Ain Issa as warplanes from the US-led coalition carried out nearly non-stop air raids.
A fragile truce agreed between the US and Russia in February had curtailed the bloodshed despite consistent allegations of violations, but the international fight against IS was excluded from the ceasefire deal.
The first of 250 members of the US special operations forces were due to arrive this week in northeast Syria to support the campaign, joining dozens of advisers already on the ground.
An SDF field commander told AFP that US ground forces were "taking part" in operations north of Raqa.
Asked about the men seen on the front line, US defence officials did not dispute that they were American special operations forces.
Observatory head Rami Abdel Rahman said IS is "concentrating 2,000 fighters along the front lines north of Raqa" to repel the SDF offensive.
"IS has prepared for this fight in recent months by digging tunnels and lining them with explosives, as well as preparing car bombs and hiding in buildings among civilians," Abdel Rahman added.